Remarkable carbon dioxide catalytic capture （CDCC） leading to solid-form carbon material via a new CVD integrated process （CVD-IP）： An alternative route for C02 sequestration-中国期刊网

摘要 Throughournewly-developed'chemicalvapordepositionintegratedprocess(CVD-IP)'usingcarbondioxide(CO2)astherawmaterialandonlycarbonsourceintroduced,CO2couldbecatalyticallyactivatedandconvertedtoanewsolid-formproduct,i.e.,carbonnanotubes(CO2-derived)ataquitehighyield(thesingle-passcarbonyieldinthesolid-formcarbon-productproducedfromCO2catalyticcaptureandconversionwasmorethan30%atasingle-passcarbon-base).Forcomparison,whenonlypurecarbondioxidewasintroducedusingtheconventionalCVDmethodwithoutintegratedprocess,nosolid-formcarbon-materialproductcouldbeformed.IntheadditionofsaturatedsteamatroomtemperatureinthefeedforCVD,thereweremuchmoreend-openingcarbonnano-tubesproduced,ataslightlyhighercarbonyield.Theseinspiringworksopenedaremarkableandalternativenewapproachforcarbondioxidecatalyticcapturetosolid-formproduct,comparingwiththatofCO2sequestration(CCS)orCO2mineralization(solidification),etc.Asaresult,therewasmuchlessbodyvolumeandalmostnogreenhouseeffectforthissolid-formcarbon-materialthanthoseofprimitivecarbondioxide.

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Remarkable carbon dioxide catalytic capture （CDCC） leading to solid-form carbon material via a new CVD integrated process （CVD-IP）： An alternative route for C02 sequestration

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Remarkable carbon dioxide catalytic capture （CDCC） leading to solid-form carbon material via a new CVD integrated process （CVD-IP）： An alternative route for C02 sequestration

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